Search for: All records

This commentary paper from the recently formed International Global Atmospheric Chemistry (IGAC) Southern Hemisphere Working Group outlines key issues in atmospheric composition research that particularly impact the Southern Hemisphere. In this article, we present a broad overview of many of the challenges for understanding atmospheric chemistry in the Southern Hemisphere, before focusing in on the most significant factors that differentiate it from the Northern Hemisphere. We present sections on the importance of biogenic emissions and fires in the Southern Hemisphere, showing that these emissions often dominate over anthropogenic emissions in many regions. We then describe how these and other factors influence air quality in different parts of the Southern Hemisphere. Finally, we describe the key role of the Southern Ocean in influencing atmospheric chemistry and conclude with a description of the aims and scope of the newly formed IGAC Southern Hemisphere Working Group. 

Abstract. Due to its remote location and extreme weather conditions, atmospheric in situmeasurements are rare in the Southern Ocean. As a result, aerosol–cloudinteractions in this region are poorly understood and remain a major source ofuncertainty in climate models. This, in turn, contributes substantially topersistent biases in climate model simulations such as the well-known positiveshortwave radiation bias at the surface, as well as biases in numericalweather prediction models and reanalyses. It has been shown in previousstudies that in situ and ground-based remote sensing measurements across theSouthern Ocean are critical for complementing satellite data sets due to theimportance of boundary layer and low-level cloud processes. These processesare poorly sampled by satellite-based measurements and are often obscured bymultiple overlying cloud layers. Satellite measurements also do not constrainthe aerosol–cloud processes very well with imprecise estimation of cloudcondensation nuclei. In this work, we present a comprehensive set of ship-basedaerosol and meteorological observations collected on the 6-weekSouthern Ocean Ross Sea Marine Ecosystem and Environment voyage(TAN1802) voyage of RV Tangaroa across the Southern Ocean, from Wellington, New Zealand, tothe Ross Sea, Antarctica. The voyage was carried out from 8 February to21 March 2018. Many distinct, but contemporaneous, data sets were collectedthroughout the voyage. The compiled data sets include measurements from arange of instruments, such as (i) meteorological conditions at the sea surfaceand profile measurements; (ii) the size and concentration of particles; (iii)trace gases dissolved in the ocean surface such as dimethyl sulfide andcarbonyl sulfide; (iv) and remotely sensed observations of low clouds. Here,we describe the voyage, the instruments, and data processing, and provide a briefoverview of some of the data products available. We encourage the scientificcommunity to use these measurements for further analysis and model evaluationstudies, in particular, for studies of Southern Ocean clouds, aerosol, andtheir interaction. The data sets presented in this study are publiclyavailable at https://doi.org/10.5281/zenodo.4060237 (Kremser et al., 2020). 

Abstract. Ambient concentrations of ice-forming particles measured during ship expeditions are collected and summarised with the aim of determining the spatial distribution and variability in ice nuclei in oceanic regions.The presented data from literature and previously unpublished data from over 23 months of ship-based measurements stretch from the Arctic to the Southern Ocean and include a circumnavigation of Antarctica. In comparison to continental observations, ship-based measurements of ambient ice nuclei show 1 to 2 orders of magnitude lower mean concentrations. To quantify the geographical variability in oceanic areas, the concentration range of potential ice nuclei in different climate zones is analysed by meridionally dividing the expedition tracks into tropical, temperate and polar climate zones. We find that concentrations of ice nuclei in these meridional zones follow temperature spectra with similar slopes but vary in absolute concentration. Typically, the frequency with which specific concentrations of ice nuclei are observed at a certain temperature follows a log-normal distribution. A consequence of the log-normal distribution is that the mean concentration is higher than the most frequently measured concentration. Finally, the potential contribution of ship exhaust to the measured ice nuclei concentration on board research vessels is analysed as function of temperature. We find a sharp onset of the influence at approximately −36 ∘C but none at warmer temperatures that could bias ship-based measurements. 

Abstract Weather and climate models are challenged by uncertainties and biases in simulating Southern Ocean (SO) radiative fluxes that trace to a poor understanding of cloud, aerosol, precipitation and radiative processes, and their interactions. Projects between 2016 and 2018 used in-situ probes, radar, lidar and other instruments to make comprehensive measurements of thermodynamics, surface radiation, cloud, precipitation, aerosol, cloud condensation nuclei (CCN) and ice nucleating particles over the SO cold waters, and in ubiquitous liquid and mixed-phase cloudsnucleating particles over the SO cold waters, and in ubiquitous liquid and mixed-phase clouds common to this pristine environment. Data including soundings were collected from the NSF/NCAR G-V aircraft flying north-south gradients south of Tasmania, at Macquarie Island, and on the RV Investigator and RSV Aurora Australis. Synergistically these data characterize boundary layer and free troposphere environmental properties, and represent the most comprehensive data of this type available south of the oceanic polar front, in the cold sector of SO cyclones, and across seasons. Results show a largely pristine environments with numerous small and few large aerosols above cloud, suggesting new particle formation and limited long-range transport from continents, high variability in CCN and cloud droplet concentrations, and ubiquitous supercooled water in thin, multi-layered clouds, often with small-scale generating cells near cloud top. These observations demonstrate how cloud properties depend on aerosols while highlighting the importance of confirmed low clouds were responsible for radiation biases. The combination of models and observations is examining how aerosols and meteorology couple to control SO water and energy budgets.